Rounds are great for jerky, but I love making top round as steak. Most people say to use marinade but I just use a dry rub. I let that sit and come to room temp with salt and pepper and some herbs on it, and heat the grill to 450. I pat it dry just before putting it on the grill. Depends on thickness but 1.5" is usually 14 minutes, 2" about 16 minutes, flipping halfway. You want it medium rare all the way through, not just in the middle, so 1 1/2" cuts are easiest.
On most top rounds, against the grain is longways, so you'll get really long slices. Medium rare all the way through, cutting it that direction in 1/4" thick slices, and you should have tender juicy steak.
This, I think I understand now. I was cutting into 3/4 x 3/4 pieces. I think what you are saying is to cut with the grain 1/4 thick, and then when I cut the other way it will be whatever but that will make it more tender?
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